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R&D: Field-free Perpendicular Magnetization Switching by Altermagnet with Collinear Spin Current

Findings provide effective method for manipulating spin currents, which is advantageous for exploration of altermagnetic spintronic devices with field-free perpendicular magnetization switching

arXiv has published an article written by M. Q. Dong, Key Laboratory of Computational Physical Sciences (Ministry of Education), Institute of Computational Physical Sciences, State Key Laboratory of Surface Physics, and Department of Physics, Fudan University, Shanghai 200433, China, Zhi-Xin Guo, State Key Laboratory for Mechanical Behavior of Materials, School of Materials Science and Engineering, Xi’an Jiaotong University, Xi’an, Shanxi 710049, China, and Xin-Gao Gong, Key Laboratory of Computational Physical Sciences (Ministry of Education), Institute of Computational Physical Sciences, State Key Laboratory of Surface Physics, and Department of Physics, Fudan University, Shanghai 200433, China.

Abstract: The generation of collinear spin current (CSC), where both the propagation direction and spin-polarized direction aligned perpendicularly to the applied charge current, is crucial for efficiently manipulating systems with perpendicular magnetic anisotropy used in high-density magnetic recording. However, the efficient generation of CSC remains a challenge. In this work, based on the symmetry analysis, we propose that CSC can be effectively generated using altermagnets when the charge current is aligned along specific directions, due to spin-dependent symmetry breaking. This proposal is supported by density functional theory (DFT) and Boltzmann transport equation (BTE) calculations on a series of altermagnetic materials, including RuO2, Mn5Si3, KRu4O8 and CuF2, where unusually large CSC is produced by the charge current along certain orientations. Furthermore, we introduce a physical quantity, the spin-splitting angle, to quantify the efficiency of CSC generated by the charge current. We find that the spin-splitting angle ranges from 0.24 to 0.57 in these altermagnets, which is significantly larger than the spin-Hall angle typically observed in the anomalous spin-Hall effect, where the spin-Hall angle is generally less than 0.1. Our findings provide an effective method for manipulating spin currents, which is advantageous for the exploration of altermagnetic spintronic devices with field-free perpendicular magnetization switching.

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